The pictures of the star come just days after her father, Jon Voight, has demanded Angelina deserved to be nominated for an Oscar.
Unbroken, a highly anticipated Second World War epic, was seen as Ange's breakthrough movie as a director.
But while the film gained three Oscar nods, including for best cinematography, Angelina missed out on a chance to win the much coveted gong.
Staring into the camera, Angelina is clearly recognisable despite the shoot taking place in 1991 - meaning the mother-of-six was 16 years old.
Her brunette hair tied up, the star looked confident and pouted for the camera as she posed wearing a black one-piece.
Practising many poses, Ange was sat on a black leather stool swivelling around as she changed position.
In a nod to her Tomb Raider days, the youngster then changed into a black PVC top and lace black leggings.
The 76-year-old added: "I think her direction is really astounding and if she wasn't my daughter I'd still say, 'I want to work for that one'."
He continued: "She's a great actor's director - the pace of the film, the size of the film. Unbelievably difficult stuff that she accomplished."
Father and daughter have both had previous Oscar success however: Jon won the best actor gong in 1978 for playing a paraplegic in Coming Home, while Angelina got 1999's best supporting actress for Girl, Interrupted.
The pictures of the star come just days after her father, Jon Voight, has demanded Angelina deserved to be nominated for an Oscar.
Unbroken, a highly anticipated Second World War epic, was seen as Ange's breakthrough movie as a director.
But while the film gained three Oscar nods, including for best cinematography, Angelina missed out on a chance to win the much coveted gong.
The 76-year-old added: "I think her direction is really astounding and if she wasn't my daughter I'd still say, 'I want to work for that one'."
He continued: "She's a great actor's director - the pace of the film, the size of the film. Unbelievably difficult stuff that she accomplished."
Father and daughter have both had previous Oscar success however: Jon won the best actor gong in 1978 for playing a paraplegic in Coming Home, while Angelina got 1999's best supporting actress for Girl, Interrupted.
Source:http://www.express.co.uk/news/showbiz/559384/Angelina-Jolie-first-photoshoot-aged-16
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